Synthesis of onion-peel nanodendritic structures with sequential functional phosphorus diversity

Chemistry : a European Journal
Nadia KatirJean Pierre Majoral

Abstract

The preparation of novel families of phosphorus-based macromolecular architectures called "onion peel" phosphorus nanodendritic systems is reported. This construct is based on the versatility of methods of synthesis using several building blocks and on the capability of these systems to undergo regioselective reactions within the cascade structure. Sustainable metal-free routes such as the Staudinger reaction or Schiff-base condensation, involving only water and nitrogen as byproducts, allow access to several dendritic macromolecules bearing up to seven different phosphorus units in their backbone, each of them featuring specific reactivity. The presence of the highly aurophilic P=N-P=S fragment enables selective ligation of Au(I) within the dendritic framework.

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Citations

May 27, 2015·Molecules : a Journal of Synthetic Chemistry and Natural Product Chemistry·Mathieu ArseneaultJean-François Morin
Apr 28, 2016·Molecules : a Journal of Synthetic Chemistry and Natural Product Chemistry·Anne-Marie Caminade, Jean-Pierre Majoral
Mar 31, 2016·Macromolecular Rapid Communications·Helena HenkeIan Teasdale
Jan 4, 2017·Macromolecular Rapid Communications·Helena HenkeIan Teasdale
Nov 4, 2015·Dalton Transactions : an International Journal of Inorganic Chemistry·Anne-Marie CaminadeJean-Pierre Majoral
May 27, 2016·Dalton Transactions : an International Journal of Inorganic Chemistry·Maria ZablockaJean-Pierre Majoral
Jul 25, 2019·Current Pharmaceutical Design·Vijay MishraNamita Giri
Apr 12, 2020·Molecules : a Journal of Synthetic Chemistry and Natural Product Chemistry·Paul Strasser, Ian Teasdale
Aug 18, 2020·Beilstein Journal of Nanotechnology·Sébastien GottisAnne-Marie Caminade
Dec 8, 2020·Drug Discovery Today·Serge MignaniJean-Pierre Majoral
Jul 3, 2021·Molecules : a Journal of Synthetic Chemistry and Natural Product Chemistry·Serge MignaniJean-Pierre Majoral
Aug 14, 2020·Bioconjugate Chemistry·Serge MignaniJean-Pierre Majoral

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