The Chemical History of a Bubble

Accounts of Chemical Research
Kenneth S SuslickHangxun Xu

Abstract

Acoustic cavitation (the growth, oscillation, and rapid collapse of bubbles in a liquid) occurs in all liquids irradiated with sufficient intensity of sound or ultrasound. The collapse of such bubbles creates local heating and provides a unique source of energy for driving chemical reactions. In addition to sonochemical bond scission and formation, cavitation also induces light emission in many liquids. This phenomenon of sonoluminescence (SL) has captured the imagination of many researchers since it was first observed 85 years ago. SL provides a direct probe of cavitation events and has provided most of our understanding of the conditions created inside collapsing bubbles. Spectroscopic analyses of SL from single acoustically levitated bubbles as well as from clouds of bubbles have revealed molecular, atomic, and ionic line and band emission riding atop an underlying continuum arising from radiative plasma processes. Application of spectrometric methods of pyrometry and plasma diagnostics to these spectra has permitted quantitative measurement of the intracavity conditions: relative peak intensities for temperature measurements, peak shifts and broadening for pressures, and peak asymmetries for plasma electron densities. The s...Continue Reading

References

Dec 10, 1987·Nature·K S Suslick, E B Flint
Oct 4, 2000·Physical Review Letters·Y T DidenkoK S Suslick
Oct 25, 2000·Physical Review. E, Statistical Physics, Plasmas, Fluids, and Related Interdisciplinary Topics·K R WeningerS J Putterman
Nov 1, 2000·Nature·Y T DidenkoK S Suslick
May 15, 2002·Physical Review Letters·George VazquezK Weninger
Mar 4, 2005·Nature·David J Flannigan, Kenneth S Suslick
Aug 11, 2005·Physical Review Letters·David J Flannigan, Kenneth S Suslick
Oct 14, 2005·Journal of the American Chemical Society·James D OxleyKenneth S Suslick
Jun 29, 2006·Physical Review Letters·David J FlanniganKenneth S Suslick
Jul 28, 2006·The Journal of Physical Chemistry. a·David J Flannigan, Kenneth S Suslick
Mar 10, 2007·Journal of the American Chemical Society·Nathan C Eddingsaas, Kenneth S Suslick
Mar 23, 1990·Science·K S Suslick
Sep 20, 1991·Science·E B Flint, K S Suslick
Oct 13, 2007·Physical Review Letters·David J Flannigan, Kenneth S Suslick
Mar 21, 2008·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·Kyuichi YasuiAtsuya Towata
Apr 9, 2008·Annual Review of Physical Chemistry·Kenneth S Suslick, David J Flannigan
Apr 30, 2009·Journal of the American Chemical Society·Hangxun XuKenneth S Suslick
Jan 6, 2010·Angewandte Chemie·Hangxun XuKenneth S Suslick
Jan 21, 2011·Ultrasonics Sonochemistry·Kenneth S SuslickHangxun Xu
Jul 21, 2011·Physical Review Letters·Brian KappusSeth Putterman
Nov 21, 2012·Chemical Society Reviews·Hangxun XuKenneth S Suslick
Jan 17, 2013·Chemical Society Reviews·Giancarlo CravottoPedro Cintas
Sep 27, 2013·Physical Chemistry Chemical Physics : PCCP·Darya RadziukKenneth Suslick
Jul 26, 2014·Physical Review Letters·A BatallerS Putterman
Nov 2, 2015·The Journal of the Acoustical Society of America·Lawrence A Crum
Oct 25, 2016·Ultrasonics Sonochemistry·Andrea ThiemannRobert Mettin
Jan 13, 2017·Topics in Current Chemistry·Jordan J Hinman, Kenneth S Suslick

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Citations

Apr 24, 2019·Chemical Communications : Chem Comm·David RoyDeborah E Crawford
Jul 14, 2020·Environmental Science and Pollution Research International·Monika JainMika Sillanpää
Mar 16, 2021·The Journal of Organic Chemistry·Hyo Na Kim, Kenneth S Suslick
Jun 23, 2021·The Journal of Organic Chemistry·R Fernando MartínezPedro Cintas
Jul 9, 2021·Langmuir : the ACS Journal of Surfaces and Colloids·Valery V Belousov, Sergey V Fedorov
Sep 4, 2021·Nanoscale·Dan SongZhibiao Wang
Nov 13, 2021·Chemical Reviews·Athanasios G AthanassiadisPeer Fischer
Sep 29, 2018·Ultrasonics Sonochemistry·Adis A TukhbatullinAkhat G Mustafin
Aug 28, 2019·Ultrasonics Sonochemistry·Jinfu LiangWeizhong Chen
Jun 19, 2019·Ultrasonics Sonochemistry·Silvia NalessoJudy Lee

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