The dependence of chlorine decay and DBP formation kinetics on pipe flow properties in drinking water distribution

Water Research
Yingying ZhaoTu-qiao Zhang

Abstract

Simultaneous chlorine decay and disinfection byproduct (DBP) formation have been discussed extensively because of their regulatory and operational significance. This study further examines chemical reaction variability in the water quality changes under various hydrodynamic conditions in drinking water distribution. The variations of kinetic constant for overall chlorine decay (kE) and trihalomethane (THM) formation were determined under stagnant to turbulent flows using three devices of different wall demand and two types of natural organic matters (NOM) in water. The results from the comparative experiments and modeling analyses show the relative importance of wall demand (kw), DBP-forming chlorine decay (kD), and other bulk demand (kb') for pipe flows of Re = 0-52500. It is found that chlorine reactivity of virgin NOM is the overriding factor. Secondly, for tap water NOM of lower reactivity, pipe flow properties (Re or u) can significantly affect kE, the THM yield (T), formation potential (Y), and the time to reach the maximum THM concentration (tmax) through their influence on kinetic ratio kD(kb'+kw). These observations, corroborating with turbidity variations during experiments, cannot be explained alone by chlorine dispe...Continue Reading

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