Transport and fate of antibiotics in a typical aqua-agricultural catchment explained by rainfall events: Implications for catchment management.

Journal of Environmental Management
Jianwei DongXinghui Xia

Abstract

Antibiotics receive many concerns since their negative environmental impacts are being revealed, especially in aqua-agricultural areas. Rainfall events are responsible for transferring excess contaminants to receiving waters. However, the understanding of antibiotics transport and fate responding to rainfall events was constrained by limited event-based data and lacking integrated consideration of dissolved and particulate forms. We developed an intensive monitoring strategy to capture responses of fourteen antibiotics to different types of rainfall events and inter-event low flow periods. Pollutant-rich suspended particles, as high as 1471 ng/g, were found in low flow periods while the very heavy rainfall events and consecutive rainfall events stimulated the release of antibiotics from eroded soil particles to river water. Therefore, these rainfall events drove radical increase of dissolved antibiotic concentration up to 592 ng/L and total flux up to 25.0 g/d. Sulfonamides were particularly sensitive to rainfall events because of their residues in manure-applied agricultural lands. Transport dynamics of most antibiotics were accretion whereas only clarithromycin exhibited a dilution pattern by concentration-discharge relations...Continue Reading

References

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Apr 8, 2010·Chemosphere·Raquel A Figueroa-DivaAllison A MacKay
Dec 27, 2012·The Science of the Total Environment·Li-Jun ZhouChang-Gui Pan
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Mar 13, 2019·The Science of the Total Environment·Xiaohui LiuWeiliang Wang
May 30, 2020·The Science of the Total Environment·James N Hitchcock

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