Ultrafast structural molecular dynamics investigated with 2D infrared spectroscopy methods

Topics in Current Chemistry
Jan Philip Kraack

Abstract

Ultrafast, multi-dimensional infrared (IR) spectroscopy has been advanced in recent years to a versatile analytical tool with a broad range of applications to elucidate molecular structure on ultrafast timescales, and it can be used for samples in a many different environments. Following a short and general introduction on the benefits of 2D IR spectroscopy, the first part of this chapter contains a brief discussion on basic descriptions and conceptual considerations of 2D IR spectroscopy. Outstanding classical applications of 2D IR are used afterwards to highlight the strengths and basic applicability of the method. This includes the identification of vibrational coupling in molecules, characterization of spectral diffusion dynamics, chemical exchange of chemical bond formation and breaking, as well as dynamics of intra- and intermolecular energy transfer for molecules in bulk solution and thin films. In the second part, several important, recently developed variants and new applications of 2D IR spectroscopy are introduced. These methods focus on (i) applications to molecules under two- and three-dimensional confinement, (ii) the combination of 2D IR with electrochemistry, (iii) ultrafast 2D IR in conjunction with diffraction...Continue Reading

References

Oct 15, 1991·Proceedings of the National Academy of Sciences of the United States of America·M H VosJ L Martin
Mar 3, 1999·Proceedings of the National Academy of Sciences of the United States of America·P HammR M Hochstrasser
Nov 28, 1994·Physical Review Letters·A Peremans, A Tadjeddine
Sep 13, 2001·Proceedings of the National Academy of Sciences of the United States of America·S WoutersenP Hamm
Sep 20, 2001·Proceedings of the National Academy of Sciences of the United States of America·M T ZanniR M Hochstrasser
Jan 12, 2002·Current Opinion in Structural Biology·M T Zanni, R M Hochstrasser
Jan 25, 2002·Analytical Chemistry·Timothy J JohnsonLaurie E Locascio
May 31, 2002·Nature·Jennifer L HerekMarcus Motzkus
Mar 11, 2003·Annual Review of Physical Chemistry·David M Jonas
Jun 27, 2003·Current Opinion in Chemical Biology·Paul Watts, Stephen J Haswell
Oct 22, 2003·Current Opinion in Structural Biology·Carl Hansen, Stephen R Quake
Jan 6, 2004·Proceedings of the National Academy of Sciences of the United States of America·Andrew Moran, Shaul Mukamel
Feb 26, 2004·Angewandte Chemie·Stéphane Chenevarin, Frédéric Thibault-Starzyk
Apr 15, 2004·Chemical Reviews·Erik T J Nibbering, Thomas Elsaesser
Aug 13, 2004·Philosophical Transactions. Series A, Mathematical, Physical, and Engineering Sciences·Fritz Keilmann, Rainer Hillenbrand
Aug 21, 2004·Proceedings of the National Academy of Sciences of the United States of America·Cathie VentalonManuel Joffre
Aug 31, 2004·The Journal of Chemical Physics·Tobias BrixnerGraham R Fleming
Sep 16, 2004·The Journal of Chemical Physics·Jens BredenbeckPeter Hamm
Mar 3, 2005·The Journal of Chemical Physics·Eric C FulmerMartin T Zanni
Mar 31, 2005·Annual Review of Physical Chemistry·Erik T J NibberingEhud Pines
May 11, 2005·Chemphyschem : a European Journal of Chemical Physics and Physical Chemistry·Wendel WohllebenMarcus Motzkus
Jul 26, 2005·Proceedings of the National Academy of Sciences of the United States of America·Yung Sam Kim, Robin M Hochstrasser
Sep 2, 2005·Proceedings of the National Academy of Sciences of the United States of America·J D EavesP L Geissler
Sep 15, 2005·Chemical Reviews·Biman Bagchi
Oct 4, 2005·Physical Review Letters·Jens BredenbeckPeter Hamm
Dec 8, 2005·The Journal of Physical Chemistry. a·Dmitry V KurochkinIgor V Rubtsov
Mar 7, 2006·Nature Reviews. Drug Discovery·Petra S Dittrich, Andreas Manz
Mar 21, 2006·Optics Letters·Sang-Hee ShimMartin T Zanni
Apr 28, 2006·The Journal of Physical Chemistry. B·Yung Sam Kim, Robin M Hochstrasser
Jun 9, 2006·Photochemical & Photobiological Sciences : Official Journal of the European Photochemistry Association and the European Society for Photobiology·Stefania AbbruzzettiJohn E T Corrie
Sep 2, 2006·Science·Valentyn I ProkhorenkoR J Dwayne Miller
Sep 13, 2006·The Journal of Chemical Physics·Sean T RobertsAndrei Tokmakoff
Oct 4, 2006·Current Opinion in Chemical Biology·Roger M Leblanc
Oct 6, 2006·The Journal of Physical Chemistry. B·Kyungwon KwakM D Fayer

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Citations

Jun 27, 2018·Topics in Current Chemistry·Jan Philip Kraack, Tiago Buckup
Dec 7, 2018·The Review of Scientific Instruments·E DenizJ Bredenbeck
Nov 29, 2017·Journal of the American Chemical Society·Daniela Kern-MichlerJens Bredenbeck
Dec 31, 2019·The Journal of Physical Chemistry Letters·Xiaoqian LiHongtao Bian
Dec 14, 2017·The Journal of Physical Chemistry Letters·Jan Philip KraackPeter Hamm
Jun 30, 2019·Journal of the American Chemical Society·Karsten Heyne, Oliver Kühn
Jan 14, 2022·The Journal of Physical Chemistry Letters·Dexia ZhouYu Fang

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